The North Atlantic Oscillation (NAO) is the major source of variability in winter atmospheric circulation in the Northern Hemisphere, with large impacts on temperature, precipitation and storm tracks, and therefore also on strategic sectors such as insurance, renewable energy production, crop yields and water management. Recent developments in dynamical methods offer promise to improve seasonal NAO predictions, but assessing potential predictability on multi-annual timescales requires documentation of past low-frequency variability in the NAO.