The atmospheric nitrous oxide mixing ratio has increased by 20% since 1750. Given that nitrous oxide is both a long-lived greenhouse gas and a stratospheric ozone-depleting substance, this increase is of global concern. However, the magnitude and geographic distribution of nitrous oxide sources, and how they have changed over time, is uncertain. A key unknown is the influence of the stratospheric circulation which brings air depleted in nitrous oxide to the surface.